Here I have created sample that will help you out.

HTML

<div>
    <asp:PlaceHolder ID="PlaceHolder1" runat="server" />
</div>

Code

protected void Page_Load(object sender, EventArgs e)
{
    if (!this.IsPostBack)
    {
        DataTable dt = this.GetData();
        StringBuilder html = new StringBuilder();
        html.Append("<table border = '1'>");
        html.Append("<tr>");
        html.Append("<th></th>");
        foreach (DataColumn column in dt.Columns)
        {
            html.Append("<th>");
            html.Append(column.ColumnName);
            html.Append("</th>");
        }
        html.Append("</tr>");
        int count = 0;
        foreach (DataRow row in dt.Rows)
        {
            html.Append("<tr>");
            html.Append("<td>");
            html.Append("<input id='rb" + count + "' type='radio' name='rb" + count + "' value='rb' /><label for='rb" + count + "'>Select</label>");
            html.Append("</td>");
            foreach (DataColumn column in dt.Columns)
            {
                html.Append("<td>");
                html.Append(row[column.ColumnName]);
                html.Append("</td>");
            }
            html.Append("</tr>");
            count++;
        }
        html.Append("</table>");
        PlaceHolder1.Controls.Add(new Literal { Text = html.ToString() });
    }
}

private DataTable GetData()
{
    DataTable dt = new DataTable();
    dt.Columns.AddRange(new DataColumn[3] { new DataColumn("Id", typeof(int)),
                        new DataColumn("Name", typeof(string)),
                        new DataColumn("Country",typeof(string)) });
    dt.Rows.Add(1, "John Hammond", "United States");
    dt.Rows.Add(2, "Mudassar Khan", "India");
    dt.Rows.Add(3, "Suzanne Mathews", "France");
    dt.Rows.Add(4, "Robert Schidner", "Russia");
    return dt;
}

VB

Protected Sub Page_Load(sender As Object, e As EventArgs)
	If Not Me.IsPostBack Then
		Dim dt As DataTable = Me.GetData()
		Dim html As New StringBuilder()
		html.Append("<table border = '1'>")
		html.Append("<tr>")
		html.Append("<th></th>")
		For Each column As DataColumn In dt.Columns
			html.Append("<th>")
			html.Append(column.ColumnName)
			html.Append("</th>")
		Next
		html.Append("</tr>")
		Dim count As Integer = 0
		For Each row As DataRow In dt.Rows
			html.Append("<tr>")
			html.Append("<td>")
			html.Append("<input id='rb" + count + "' type='radio' name='rb" + count + "' value='rb' /><label for='rb" + count + "'>Select</label>")
			html.Append("</td>")
			For Each column As DataColumn In dt.Columns
				html.Append("<td>")
				html.Append(row(column.ColumnName))
				html.Append("</td>")
			Next
			html.Append("</tr>")
			count += 1
		Next
		html.Append("</table>")
		PlaceHolder1.Controls.Add(New Literal() With { _
			Key .Text = html.ToString() _
		})
	End If
End Sub

Private Function GetData() As DataTable
	Dim dt As New DataTable()
	dt.Columns.AddRange(New DataColumn(2) {New DataColumn("Id", GetType(Integer)), New DataColumn("Name", GetType(String)), New DataColumn("Country", GetType(String))})
	dt.Rows.Add(1, "John Hammond", "United States")
	dt.Rows.Add(2, "Mudassar Khan", "India")
	dt.Rows.Add(3, "Suzanne Mathews", "France")
	dt.Rows.Add(4, "Robert Schidner", "Russia")
	Return dt
End Function

Screenshot