Hi rani,
Check this example. Now please take its reference and correct your code.
Database
I have made use of the following table Customers with the schema as follows.

I have already inserted few records in the table.

You can download the database table SQL by clicking the download link below.
Download SQL file
HTML
<html xmlns="http://www.w3.org/1999/xhtml">
<head runat="server">
    <title>Inline Editing in AngularJS</title>
    <link rel="stylesheet" href="https://maxcdn.bootstrapcdn.com/bootstrap/3.3.2/css/bootstrap.min.css" />
    <script type="text/javascript" src="https://ajax.googleapis.com/ajax/libs/angularjs/1.6.9/angular.min.js"></script>
    <script type="text/javascript">
        var app = angular.module('MyApp', []);
        app.controller('MyController', function ($scope, $http, $window) {
            $scope.Customers = [];
            PopulateCustomers($scope, $http);
            $scope.EditCustomer = function (id) {
                for (var i = 0; i < $scope.Customers.length; i++) {
                    if ($scope.Customers[i].Id == id) {
                        $scope.Customers[i].EditMode = true;
                    } else {
                        $scope.Customers[i].EditMode = false;
                    }
                }
            }
            $scope.UpdateCustomer = function (customer) {
                var data = { id: customer.Id, name: customer.Name, country: customer.Country };
                $http.post("Default.aspx/UpdateCustomer", JSON.stringify(data), { headers: { 'Content-Type': 'application/json'} })
                .then(function (response) {
                    PopulateCustomers($scope, $http);
                });
            }
            $scope.DeleteCustomer = function (customer) {
                if ($window.confirm("Do you want to delete customer " + customer.Name + " ?")) {
                    var data = { id: customer.Id };
                    $http.post("Default.aspx/DeleteCustomer", JSON.stringify(data), { headers: { 'Content-Type': 'application/json'} })
                    .then(function (response) {
                        PopulateCustomers($scope, $http);
                    });
                }
            }
            $scope.CancelEdit = function (customer) {
                for (var i = 0; i < $scope.Customers.length; i++) {
                    $scope.Customers[i].EditMode = false;
                }
            }
        });
        function PopulateCustomers($scope, $http) {
            $http.post("Default.aspx/GetCustomers", { headers: { 'Content-Type': 'application/json'} })
            .then(function (response) {
                $scope.Customers = eval(response.data.d);
            });
        }
    </script>
</head>
<body>
    <form id="form1" runat="server">
    <div ng-app="MyApp" ng-controller="MyController">
        <table class="table table-striped table-bordered">
            <thead>
                <tr>
                    <th>Name</th>
                    <th>Country</th>
                    <th>Action</th>
                </tr>
            </thead>
            <tbody>
                <tr ng-repeat="customer in Customers">
                    <td>
                        <span ng-show="!customer.EditMode">{{customer.Name}}</span>
                        <input class="form-control" type="text" ng-model="customer.Name" ng-show="customer.EditMode" />
                    </td>
                    <td>
                        <span ng-show="!customer.EditMode">{{customer.Country}}</span>
                        <input class="form-control" type="text" ng-model="customer.Country" ng-show="customer.EditMode" />
                    </td>
                    <td>
                        <div ng-show="!customer.EditMode">
                            <button type="button" class="btn btn-primary btn-sm glyphicon glyphicon-edit" ng-click="EditCustomer(customer.Id)">
                                 Edit</button>
                            <button type="button" class="btn btn-danger btn-sm glyphicon glyphicon-remove" ng-click="DeleteCustomer(customer)">
                                 Delete</button>
                        </div>
                        <div ng-show="customer.EditMode">
                            <button type="button" class="btn btn-success btn-sm glyphicon glyphicon-ok" ng-click="UpdateCustomer(customer)">
                                 Update</button>
                            <button type="button" class="btn btn-default btn-sm glyphicon glyphicon-erase" ng-click="CancelEdit(customer)">
                                 Cancel</button>
                        </div>
                    </td>
                </tr>
            </tbody>
        </table>
    </div>
    </form>
</body>
</html>
Namespaces
C#
using System.Collections.Generic;
using System.Configuration;
using System.Data.SqlClient;
using System.Web.Script.Serialization;
using System.Web.Services;
VB.Net
Imports System.Collections.Generic
Imports System.Configuration
Imports System.Data.SqlClient
Imports System.Web.Script.Serialization
Imports System.Web.Services
Code
C#
[WebMethod]
public static string GetCustomers()
{
    List<object> customers = new List<object>();
    string sql = "SELECT * FROM Customers";
    using (SqlConnection conn = new SqlConnection())
    {
        conn.ConnectionString = ConfigurationManager.ConnectionStrings["constr"].ConnectionString;
        using (SqlCommand cmd = new SqlCommand(sql))
        {
            cmd.Connection = conn;
            conn.Open();
            using (SqlDataReader sdr = cmd.ExecuteReader())
            {
                while (sdr.Read())
                {
                    customers.Add(new
                    {
                        Id = sdr["CustomerId"],
                        Name = sdr["Name"],
                        Country = sdr["Country"]
                    });
                }
            }
            conn.Close();
        }
        return (new JavaScriptSerializer().Serialize(customers));
    }
}
[WebMethod]
public static void UpdateCustomer(int id, string name, string country)
{
    string sql = "UPDATE Customers SET Name = @Name, Country = @Country WHERE CustomerId = @Id";
    using (SqlConnection con = new SqlConnection())
    {
        con.ConnectionString = ConfigurationManager.ConnectionStrings["constr"].ConnectionString;
        using (SqlCommand cmd = new SqlCommand(sql))
        {
            cmd.Connection = con;
            cmd.Parameters.AddWithValue("@Id", id);
            cmd.Parameters.AddWithValue("@Name", name);
            cmd.Parameters.AddWithValue("@Country", country);
            con.Open();
            cmd.ExecuteNonQuery();
            con.Close();
        }
    }
}
[WebMethod]
public static void DeleteCustomer(int id)
{
    string sql = "DELETE FROM Customers WHERE CustomerId = @Id";
    using (SqlConnection con = new SqlConnection())
    {
        con.ConnectionString = ConfigurationManager.ConnectionStrings["constr"].ConnectionString;
        using (SqlCommand cmd = new SqlCommand(sql))
        {
            cmd.Connection = con;
            cmd.Parameters.AddWithValue("@Id", id);
            con.Open();
            cmd.ExecuteNonQuery();
            con.Close();
        }
    }
}
VB.Net
<WebMethod()>
Public Shared Function GetCustomers() As String
    Dim customers As List(Of Object) = New List(Of Object)()
    Dim sql As String = "SELECT * FROM Customers"
    Using conn As SqlConnection = New SqlConnection()
        conn.ConnectionString = ConfigurationManager.ConnectionStrings("constr").ConnectionString
        Using cmd As SqlCommand = New SqlCommand(sql)
            cmd.Connection = conn
            conn.Open()
            Using sdr As SqlDataReader = cmd.ExecuteReader()
                While sdr.Read()
                    customers.Add(New With {
                        .Id = sdr("CustomerId"),
                        .Name = sdr("Name"),
                    .Country = sdr("Country")
                    })
                End While
            End Using
            conn.Close()
        End Using
        Return (New JavaScriptSerializer().Serialize(customers))
    End Using
End Function
<WebMethod()>
Public Shared Sub UpdateCustomer(ByVal id As Integer, ByVal name As String, ByVal country As String)
    Dim sql As String = "UPDATE Customers SET Name = @Name, Country = @Country WHERE CustomerId = @Id"
    Using con As SqlConnection = New SqlConnection()
        con.ConnectionString = ConfigurationManager.ConnectionStrings("constr").ConnectionString
        Using cmd As SqlCommand = New SqlCommand(sql)
            cmd.Connection = con
            cmd.Parameters.AddWithValue("@Id", id)
            cmd.Parameters.AddWithValue("@Name", name)
            cmd.Parameters.AddWithValue("@Country", country)
            con.Open()
            cmd.ExecuteNonQuery()
            con.Close()
        End Using
    End Using
End Sub
<WebMethod()>
Public Shared Sub DeleteCustomer(ByVal id As Integer)
    Dim sql As String = "DELETE FROM Customers WHERE CustomerId = @Id"
    Using con As SqlConnection = New SqlConnection()
        con.ConnectionString = ConfigurationManager.ConnectionStrings("constr").ConnectionString
        Using cmd As SqlCommand = New SqlCommand(sql)
            cmd.Connection = con
            cmd.Parameters.AddWithValue("@Id", id)
            con.Open()
            cmd.ExecuteNonQuery()
            con.Close()
        End Using
    End Using
End Sub
Screenshot
